CHAPTER 20  ANTIMICROBIAL DRUGS

 

Chemotherapeutic drugs (chemotherapy) combat disease in the body, whether it is caused by a pathogenic microbe or something else (cancer)

 

An antimicrobial drug is a chemical that destroys pathogenic microbes with minimal damage to the tissues of the host—this is selective toxicity.

 

Antibiotic---this is specifically a chemical invented by one microbe to work against other microbes

 

Synthetic---prepared in the laboratory, no microbe involved

 

Semisynthetic-----the original antibiotic is changed or modified in the lab

 

 

HISTORY OF CHEMOTHERAPY

 

1. Although chemotherapy with natural products such as herbs can be traced back far in the history of man, Paul Ehrlich is given credit for the birth of modern chemotherapy. He set out to create a treatment for syphilis that would cure the disease more reliably and with less harm to the patient than existing treatments, which involved the use of mercury. His discovery was Salvarsan, a modified form of arsenic. It was first called Compound 606, because Ehrlich had tried 605 compounds before it which did not work.

 

2. In 1928, Alexander Fleming observed that a mold which had appeared as a contaminant in a Petri dish of bacteria had prevented bacterial growth in the area surrounding it. The mold was identified as Penicillium notatum. Fleming regarded his discovery as a curiosity and made little effort to develop it.

 

3. In 1935, Domagk and Trefoil discovered and developed the antimicrobial properties of a synthetic red dye called prontosil. Living cells change prontosil into sulfanilamide, which is antimicrobial. At first, the sulfas were used as a powder to dust on wounds. Later they were developed into systemic drugs, and derivatives are widely used today. Since sulfas are synthetic, they are not true antibiotics.

 

4. In 1940, Florey and Chain worked with penicillin, the active compound in Fleming’s discovery, and brought it to clinical trials. At that time, it was extremely difficult to produce penicillin, but it showed promise. The work was moved to the US because of the danger of bombing in England, and by the end of World War II penicillin was becoming readily available. It worked like magic and was called the “wonder drug,” with its best effect against gram-positive bacteria.

 

5. Selman Waksman soon discovered streptomycin, which worked very well against gram-negative bacteria. At that point, many scientists believed (mistakenly) that we had won the war against bacteria.

 

 

SOURCES OF ANTIBIOTICS

 

Most antibiotics come from soil bacteria. A great number of the antibiotics that are discovered are so toxic that while they kill all known bacteria, they also kill the patient. Only a small percentage can be developed for use in treating disease. Some organisms that produce antibiotics are:

 

1. Members of the genus Streptomyces (bacteria)--more than half our antibiotics

2. Members of the genus Bacillus (bacteria)

3. Members of the genus Cephalosporium (fungus)

4. Members of the genus Penicillium (fungus)

 

                    TABLE  20.1  P. 582

 

 

SPECTRUM OF ANTIMICROBIAL ACTIVITY

 

The goal that must always be kept in mind is that the antimicrobial must cause more harm to the pathogen than to the host.  This is called selective toxicity.  We have had our greatest success with antibacterial antibiotics, since there are a number of things that are different in procaryotic bacterial cells from the eucaryotic cells of the host. These differences make it relatively easy to target the pathogen and spare the host. Attacking the eucaryotic cells of fungi, helminths,  and protozoa, and the host cells that viruses have invaded is more difficult.

 

Antimicrobials may work against only certain microbes. They can be:

·         Antibacterial

·         Antifungal

·         Antiviral

·         Antiprotozoal

 

The spectrum of activity is the range of different microbes a drug is able to work against.  Narrow-spectrum means that the drug works best against only a certain group or type; broad-spectrum drugs work against a wider range of microbes. If the drug works against bacteria, a broad-spectrum drug would probably do well against both gram-positive and gram-negative organisms. A narrow-spectrum drug would work only against one or the other, or possibly an even narrower group.

 

An ideal antimicrobial would have more effect against pathogens and less on the normal flora of the body. Unfortunately, this is not always possible.

 

 

ACTION OF ANTIMICROBIAL DRUGS

 

Antimicrobial drugs are either   ---cidal, which means they actually kill the pathogens, or

 ----static, which means they slow or prevent reproduction. In either case, the defenses of the host will also be needed.

 

1. inhibition of cell wall synthesis—since this attacks the cell wall, these drugs have little effect on host cells, which do not contain peptidoglycan. Penicillins, cephalosporins, bacitracin, and vancomycin act in this way. These work best on gram-positive bacteria.

 

2. Inhibition of protein synthesis---since ribosomes of procaryotic cells are slightly different from those of eucaryocytes, they can be used as a target. Chloramphenicol, erythromycin, streptomycin, gentamicin, and the tetracyclines act in this way.

 

3. Injury to the plasma membrane—this is a mode of action of both some antibacterials and some antifungals. Antifungals are able to work mostly against fungus cell membranes because they contain ergosterol instead of cholesterol. However, these antibiotics are potentially quite toxic to the host. Examples are the polymixins,  and antifungals such as amphotericin B, miconazole, and ketoconazole.

 

4. Inhibition of nucleic acid synthesis---selective toxicity varies, but these interfere with DNA replication and transcription. Rifampin and the quinolones are examples.

 

5. Inhibiting the synthesis of essential metabolites---the sulfas and trimethoprim work this way. They interfere with the pathway by which bacteria synthesize folic acid. Since humans produce folic acid by a different pathway, these drugs have less effect on human cells.

 

 

 

 

ANTIBACTERIALS:

Inhibitors of Cell Wall Synthesis:

     Natural penicillins—action depends on a part of the molecule called the β-lactam ring; resistant bacteria produce penicillinase, an enzyme which breaks down the β-lactam ring

     Semisynthetic penicillins

  Penicillinase-resistant penicillins—not inactivated by penicillinase—methicillin

     Extended-spectrum penicillins—broader spectrum—ampicillin, amosicillin

     Penicillins plus β-lactamase inhibitors—these include clavulanic acid, which prevents damage to β-lactam ring—augmentin

     Cephalosporins—structure & mode of action similar to penicillins

     Bacitracin—polypeptide antibiotic used only topically

     Vancomycin—inhibits peptidoglycan synthesis—relatively toxic but may be only drug that works against some strains of Staphylococcus aureus

 

Antimycobacterial Antibiotics:

     Isoniazid—believed to inhibit synthesis of mycolic acid

     Ethambutol—inhibits incorporation of mycolic acid into cell wall

Inhibitors of Protein Synthesis:

     Chloramphenicol—broad spectrum and can be synthesized chemically (doesn’t have to be made by a microbe)--used only when absolutely necessary due to potential for aplastic anemia

     Aminoglycosides—streptomycin, neomycin, gentamicin—may be toxic to auditory nerve or kidneys

     Tetracyclines—broad spectrum, effective against chlamydias & rickettsias—tetracycline, oxytetracycline, chlortetracycline,doxycycline

     Macrolides—erythromycin, clarithromycin—used to treat infections due to bacteria resistant to penicillins

     Streptogramins—developed to combat resistance to vancomycin—synercid

     Oxazolidinones—new synthetic antibiotics which may be effective abainst MRSA

 

Injury to the Plasma Membrane

     Polymixin B—used topically, very effective against gram-negative bacteria

 

 

Inhibitors of Nucleic Acid Synthesis

  Rifamycins—used to treat tuberculosis, inhibits synthesis of mRNA—rifampin

     Quinolones & Fluoroquinolenes—nalidixic acid was the first quinolone, Cipro is best known fluoroquinolone

 

Competetive Inhibitors of the Synthesis of Essential Metabolites

     Sulfonamides—sulfa drugs—block synthesis of folic acid, a precursor to nucleic acids—trimethoprim & sulfamethoxazole in combination

 

ANTIFUNGALS

Selective toxicity is a bigger problem because fungi  are eukaryotic cells. One difference is that they use ergosterol in place of cholesterol in their plasma membranes, so that is one area that antifungals can attack. Fungal cell walls are another target. Overall, antifungals are more toxic to the patient that antibacterials, and some of them require frequent test to monitor possible liver damage.

     Topical antifungals—miconazole, tolnaftate, undecylenic acid

     Systemic antifungals—amphotericin B, ketoconazole, fluconazole, terbinafine, griseofulvin

 

 

ANTIVIRALS

Antivirals are few & far between. Since viruses invade cells and use cellular mechanisms for replication of nucleic acid & protein synthesis, selective toxicity is a major problem. There are a few antivirals, and many of these are effective only against retroviruses, the group that includes HIV.

     Influenza—amantadine, Tamiflu, Relenza

     Herpes—acyclovir, ribovirin

    

 

ANTIPROTOZOAL & ANTIHELMINTHIC

    Antiprotozoals include quinine, chloroquine, quinacrine, metronidazole

     Antihelminthics include niclosamide, praziquantel, mebendazole, alendazole, ivermectin

         

                                                             TABLE 20.3  P. 587 - 590

 

 

TESTS TO GUIDE CHEMOTHERAPY    

 

Although in many cases chemotherapy is begun by guessing which drug might be effective, tests to determine effectiveness are sometimes used. This might be necessary when drug resistance is a problem, or when the patient has not responded to the first medication.

 

1. The Kirby-Bauer diffusion (disk diffusion) method—After inoculating the trouble-making organism onto an agar plate, discs containing various antibiotics are applied to the surface and zones of inhibition are observed.

 

2. The E test—this determines the minimal inhibitory concentration (MIC). The lower the concentration that is effective, the better the chance for good results in a patient. A plastic-coated strip contains a gradient of antibiotic concentrations and can be read after incubation.

 

3. Broth dilution tests---this is another way to determine the minimum inhibitory concentration that is effective. This involves use of a series of broth cultures, each containing a different concentration of the antibiotic. Although more complicated, this test is very accurate and also determines whether the drug is bacteriostatic or bacteriocidal.

 

 

 

EFFECTIVENESS OF CHEMOTHERAPEUTIC AGENTS

 What do bacteria do that makes them resistant to an antibiotic?

 

1. Microbes release an enzyme that modifies or destroys the antibiotic. Penicillinase is an example of this.

 

2. Something about the microbe changes and makes it difficult or impossible for the antibiotic to penetrate into the bacteria. This often is a change in the outer membrane.

 

3. The microbe develops a way to pump out the antibiotic so fast it does little harm. Many organisms can pump out tetracyclines, for example.

 

4. Microbe develops an alternate chemical reaction to the one the antibiotic blocks.

 

5. Microbe may make a slight change in whatever cell component the antibiotic attacks.

 

Many of these changes are due to random mutations. Once even one microbe becomes resistant, it passes the resistance on. If only microbes that are resistant survive, the entire population of microbes soon becomes resistant.

 

Another major problem with resistance is that the genes that make an organism resistant are often carried on a plasmid. The R plasmids are often shared among bacteria, increasing the resistance problem.

 

Many bacterial diseases are now very commonly resistant to antibiotics, and there are strains of pathogenic bacteria that are resistant to all known antibiotics.